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Publications


54. Magnetic Archimedean Tessellations in Metal-Organic Frameworks

H. Chen, L. Voigt, M. Kubus, D. Mihrin, S. Mossin, R. W. Larsen, S. Kegnæs, S. Piligkos, K. S. Pedersen,
J. Am. Chem. Soc. 2021, 143, 14041


53. Emergent magnetic behavior in the frustrated Yb3Ga5O12 garnet

L. Ø. Sandberg, R. Edberg, I.-M. B. Bakke, K. S. Pedersen, M. C. Hatnean, G. Balaskrishnan, L. Mangin-Thro, A. Wildes, B. Fåk, G. Ehlers, G. Sala, P. Henelius, K. Lefmann, P. P. Deen,
Phys. Rev. B, 2021, 104, 064425


52. Zero-valent metals in metal-organic frameworks: fac-M(CO)3(pyrazine)3/2

L. Voigt, R. W. Larsen, M. Kubus, K. S. Pedersen,
Chem. Commun. 2021, 57, 3861.


51. Island formation of Er(trensal) single-ion magnets on graphene observed on the micrometer scale

J. Dreiser, C. Wäckerlin, M. Buzzi, K. S. Pedersen, J. Bendix,
RSC Advances, 2021, 11, 9421.


50. Structural characterization and magnetic properties of chromium jarosite KCr3(OD)6(SO4)2

S. Janas, M. B. Sørensen, A. B. A. Andersen, M. Juelsholt, M. Böhm, K. S. Pedersen, K. M. Ø. Jensen, K. Lefmann, U. G. Nielsen,
Phys. Chem. Chem. Phys. 2020, 22, 25001.


49. Molecule-based metal-organic magnets with large room-temperature coercivity and critical temperature up to 242°C

P. Perlepe, I. Oyarzabal, A. Mailman, M. Yquel, I. Dovgaliuk, M. Platunov, M. Rouzières, Ph. Negrier, D. Mondieig, E. A. Suturina, M.-A. Dourges, S. Bonhommeau, R. Musgrave, K. S. Pedersen, D. Chernyshov, F. Wilhelm, A. Rogalev, C. Mathonière, R. Clérac,
Science, 2020, 370, 587.


48. Chemical engineering of quasicrystal approximants in lanthanide-based coordination solids

L. Voigt, M. Kubus, K. S. Pedersen,
Nat. Commun. 2020, 11, 4705.


47. Ligand field-actuated redox-activity of acetylacetonate

M. G. Vinum, L. Voigt, S. H. Hansen, C. Bell, K. M. Clark, R. W. Larsen, K. S. Pedersen,
Chem. Sci. 2020, 11, 8267.


46. Coercive Fields Above 6 T in Two Cobalt(II)-Radical Chain Compounds

X. Liu, X. Feng, K. R. Meihaus, X. Meng, Y. Zhang, L. Li, J.-L. Liu, K. S. Pedersen, L. Keller, W. Shi, Y.-Q. Zhang, P. Cheng, J. R. Long,
Angew. Chem. Int. Ed. 2020, 59, 10610.


45. Access to Heteroleptic Fluorido-Cyanido Complexes with a Large Magnetic Anisotropy via Fluoride Abstraction

J.-L. Liu, K. S. Pedersen, S. M. Greer, I. Oyarzabal, A. Mondal, S. Hill, F. Wilhelm, A. Rogalev, A. Tressaud, E. Durand, J. R. Long, R. Clérac,
Angew. Chem. Int. Ed. 2020, 59, 10306.


44. A Redox-Innocent Uranium(IV)-Quinoid Metal-Organic Framework

V. E. Refn, M. Kubus, S. Mossin, R. W. Larsen, K. S. Pedersen,
ACS Omega, 2020, 5, 3462.


43. Pentagonal-bipyramidal acetonitrile complexes of the lanthanide(II) iodides

M. Kubus, L. Voigt, K. S. Pedersen,
Inorg. Chem. Commun. 2019, 114, 107819.


42. Evidence for Non-Innocence of a B-Diketonate Ligand (“HOT” paper)

M. G. Vinum, L. Voigt, C. Bell, D. Mihrin, R. W. Larsen, K. M. Clark, K. S. Pedersen,
Chem. Eur. J. 2019, 26, 2143


41. [UF6]2−: A Molecular Hexafluorido Actinide(IV) Complex with Compensating Spin and Orbital Magnetic Moments (“HOT” paper)

K. S. Pedersen, K. R. Meihaus, A. Rogalev, F. Wilhelm, D. Aravena, M. Amoza, E. Ruiz, J. R. Long, J. Bendix, R. Clérac,
Angew. Chem. Int. Ed. 2018, 58, 15650.


40. Formation of the layered conductive magnet CrCl2(pyrazine)2 through redox-active coordination chemistry

K. S. Pedersen, P. Perlepe, M. Aubrey, D. N. Woodruff, S. Reyes-Lillo, A. Reinholdt, L. Voigt, Z. Li, K. Borup. M. Rouzieres, D. Samohvalov, F. Wilhelm, A. Rogalev, J. Neaton, J. R. Long, R. Clérac,
Nat. Chem. 2018, 10, 1056.


39. Coherent Manipulation of a Molecular Ln-Based Nuclear Qudit Coupled to an Electron Qubit

R. Hussain, G. Allodi, A. Chiesa, E. Garlatti, D. Mitcov, A. Konstantatos, K. S. Pedersen, R. De Renzi, S. Piligkos, S. Carretta,
J. Am. Chem. Soc. 2018, 140, 9814.


38. Field-induced single molecule magnet behaviour in ideal trigonal antiprismatic cobalt(II) complexes: precise geometrical control by a hydrogen-bonded rigid metalloligand

R. Mitsuhashi, K. S. Pedersen, T. Ueda, T. Suzuki, J. Bendix, M. Mikuriya,
Chem. Commun. 2018, 54, 8869.


37. Cr(pyrazine)2(OSO2CH3)2: A two-dimensional coordination polymer with an antiferromagnetic ground state

P. Perlepe, I. Oyarzabal, K. S. Pedersen, P. Negrier, D. Mondieig, M. Rouzieres, E. A. Hillard, F. Wilhelm, A. Rogalev, E. A. Suturina, C. Mathonière, R. Clérac,
Polyhedron, 2018, 153, 248.


36. Chemical tunnel-splitting-engineering in a dysprosium-based molecular nanomagnet

M. A. Sørensen, U. B. Hansen, M. Perfetti, K. S. Pedersen, E. Bartolomé, G. G. Simeoni, H. Mutka, S. Rols, M. Jeong, I. Zivkovic, M. Retuerto, A. Arauzo, J. Bartolomé, S. Piligkos, H. Weihe, L. H. Doerrer, J. van Slageren, H. M. Rønnow, K. Lefmann, J. Bendix,
Nat. Commun. 2018, 9, 1292.


35. Rational Self-Assembly of Tricobalt Extended Metal Atom Chains and [MF6]2– Building Blocks into One-Dimensional Coordination Polymers

M. Cortijo, V. Bulicanu, K. S. Pedersen, M. Rouzières, J. Bendix, R. Clérac, E. A. Hillard,
Eur. J. Inorg. Chem. 2018, 320.


34. [OsF6]x–: Molecular Models for Spin-Orbit Entangled Phenomena

K. S. Pedersen, D. N. Woodruff, S. K. Singh, A. Tressaud, E. Durand, M. Atanasov, P. Perlepe, K. Ollefs, F. Wilhelm, C. Mathonière, F. Neese, A. Rogalev, J. Bendix, R. Clérac,
Chem. Eur. J. 2017, 23, 11244.


33. Multifaceted magnetization dynamics in the mononuclear complex [ReIVCl4(CN)2]2–

X. Feng, J.-L. Liu, K. S. Pedersen, J. Nehrkorn, A. Schnegg, K. Holldack, J. Bendix, M. Sigrist, H. Mutka, D. Samohvalov, D. Aguilà, M.-L. Tong, J. R. Long, R. Clérac,
Chem. Commun. 2016, 52, 12905..


32. Iridates from the molecular side

K. S. Pedersen, J. Bendix, A. Tressaud, E. Durand, H. Weihe, Z. Salman, T. J. Morsing, D. N. Woodruff, Y. Lan, W. Wernsdorfer, C. Mathonière, S. Piligkos, S. I. Klokishner, S. I. Ostrovsky, K. Ollefs, F. Wilhelm, A. Rogalev, R. Clérac,
Nat. Commun. 2016, 7, 12195.


31. Spin Crossover in Fe(II) Complexes with N4S2 Coordination

A. Arroyave, A. Lennartson, A. Dragulescu-Andrasi, K. S. Pedersen, S. Piligkos, S. A. Stoian, S. M. Greer, O. Hietsoi, H. Phan, S. Hill, C. J. McKenzie, M. Shatruk,
Inorg. Chem. 2016, 55, 5904.


30. Toward 4f Single-Ion Magnet Qubits

K. S. Pedersen, A.-M. Ariciu, S. McAdams, F. Tuna, J. Dreiser, H. Weihe, J. Bendix, S. Piligkos
J. Am. Chem. Soc., 2016, 138, 5801.


29. Out-of-plane Alignment of Er(trensal) Easy Magnetization Axes Using Graphene

J. Dreiser, G. E. Pacchioni, F. Donati, L. Gragnaniello, A. Cavallin, K. S. Pedersen, J. Bendix, B. Delley, M. Pivetta, S. Rusponi, H. Brune,
ACS Nano, 2016, 10, 2887.


28. Cyanide Single-Molecule Magnets Exhibiting Solvent Dependent Reversible “On” and “Off” Exchange Bias Behavior

D. Pinkowicz, H. I. Southerland, C. Avendano, A. Prosvirin, C. Sanders, W. Wernsdorfer, K. S. Pedersen, J. Dreiser, R. Clérac, J. Nehrkorn, G. G. Simeoni, A. Schnegg, K. Holldack, K. R. Dunbar,
J. Am. Chem. Soc. 2015, 137, 14406.


27. One-dimensional coordination polymers of [Co3(dpa)4]2+ and [MF6]2– (M = ReIV, ZrIV, SnIV)

V. Bulicanu, K. S. Pedersen, M. Rouzières, J. Bendix, P. Dechambenoit, R. Clérac, E. A. Hillard,
Chem. Commun. 2015, 51, 17748.


26. Design of Single-Molecule Magnets: Insufficiency of the Anisotropy Barrier as the Sole Criterion

K. S. Pedersen, J. Dreiser, H. Weihe, R. Sibille, H. V. Johannesen, M. A. Sørensen, B. E. Nielsen, M. Sigrist, H. Mutka, S. Rols, J. Bendix, S. Piligkos,
Inorg. Chem. 2015, 54, 7600.


25. Magnetic and magnetocaloric properties of an unusual family of carbonate-panelled [LnIII6ZnII2] cages

W. Sethi, S. Sanz, K. S. Pedersen, M. A. Sørensen, G. S. Nichol, G. Lorusso, M. Evangelisti, E. K. Brechin, S. Piligkos,
Dalton Trans. 2015, 44, 10315.


24. Fluoride coordination chemistry in molecular and low-dimensional magnetism

K. S. Pedersen, M. A. Sørensen, J. Bendix,
Coord. Chem. Rev. 2015, 299, 1.


23. Zero-Field Splitting in {MnIII33-O)} Core Single-Molecule Magnets Investigated by Inelastic Neutron Scattering and High-Field Electron Paramagnetic Resonance Spectroscopy

M. Sigrist P. L. W. Tregenna-Piggott, K. S. Pedersen, M. A. Sørensen, A.-L. Barra, J. Hauser, S.-X. Liu, S. Decurtins, H. Mutka, J. Bendix,
Eur. J. Inorg. Chem. 2015, 2683.


22. [CrIII8MII6]12+ Coordination Cubes (MII = Cu, Co)

S. Sanz, H. O’Connor, E. M. Pineda, K. S. Pedersen, G. S. Nichol, O. Mønsted, H. Weihe, S. Piligkos, E. J. L. McInnes, P. Lusby, E. K. Brechin,
Angew. Chem. Int. Ed. 2015, 54, 6761.


21. Magnetic properties of ultra-small goethite nanoparticles

E. Brok, C. Frandsen, D. E. Madsen, H. Jacobsen, J. O. Birk, K. Lefmann, J. Bendix, K. S. Pedersen, C. B. Boothroyd, A. A. Berhe, G. G. Simeoni, S. Mørup,
J. Phys. D: Appl. Phys. 2014, 47, 365003.


20. Exchange Interaction of Strongly Anisotropic Tripodal Erbium Single-Ions Magnets with Metallic Surfaces

J. Dreiser, C. Wäckerlin, Md. E. Ali, C. Piamonteze, F. Donati, A. Singha, K. S. Pedersen, S. Rusponi, J. Bendix, P. M. Oppeneer, T. A. Jung, H. Brune,
ACS Nano, 2014, 8, 4662.


19. Single-molecule magnet engineering: building-block approaches

K. S. Pedersen, J. Bendix, R. Clérac,
Chem. Commun. 2014, 50, 4396.


18. Magnetic Interactions through Fluoride; Magnetic and Spectroscopic Characterization of Discrete, Linearly Bridged [MnIII2(μ-F)F4(Me3tacn)2](PF6)

K. S. Pedersen, M. Sigrist, H. Weihe, A. Bond, C. A. Thuesen, K. P. Simonsen, T. Birk, H. Mutka, A.-L. Barra, J. Bendix,
Inorg. Chem. 2014, 53, 5013


17. Fluoride-Bridged {GdIII3MIII2} (M = Cr, Fe, Ga) Molecular Refrigerants

K. S. Pedersen, G. Lorusso, J. J. Morales, T. Weyhermüller, S. Piligkos, S. K. Singh, D. Larsen, M. Schau-Magnussen, G. Rajaraman, M. Evangelisti, J. Bendix,
Angew. Chem. Int. Ed. 2014, 53, 2394


16. Modifying the properties of 4f single-ion magnets by peripheral ligand functionalization

K. S. Pedersen, L. Ungur, M. Sigrist, A. Sundt, M. Schau-Magnussen, V. Vieru, H. Mutka, S. Rols, H. Weihe, O. Waldmann, L. F. Chibotaru, J. Bendix, J. Dreiser,
Chem. Sci. 2014, 5, 1650.


15. [ReF6]2–: A Robust Module for the Design of Molecule-Based Magnetic Materials

K. S. Pedersen, M. Sigrist, M. A. Sørensen, A.-L. Barra, T. Weyhermüller, S. Piligkos, C. Aa. Thuesen, M. G. Vinum, H. Mutka, H. Weihe, R. Clérac, J. Bendix,
Angew. Chem. Int. Ed. 2014, 53, 1351


14. Angular dependence of the exchange interaction in fluoride-bridged GdIII–CrIII complexes.

S. K. Singh (equal contribution), K. S. Pedersen (equal contribution), M. Sigrist, C. Aa. Thuesen, M. Schau-Magnussen, H. Mutka, S. Piligkos, H. Weihe, G. Rajaraman, J. Bendix,
Chem. Commun. 2013, 49, 5583.


13. XMCD Study of the Magnetic Exchange Coupling in a Fluoride-Bridged Dy-Cr Molecular Cluster

J. Dreiser, C. Piamonteze, F. Nolting, K. S. Pedersen, J. Bendix, S. Rusponi, H. Brune,
J. Korean Phys. Soc. 2013, 62, 1368.


12. Three-Axis Anisotropic Exchange Interactions in the Single-Molecule Magnets NEt4[MnIII2(5-Brsalen)2(MeOH)2MIII(CN)6] (M = Ru, Os)

J. Dreiser, K. S. Pedersen, A. Schnegg, K. Holldack, J. Nehrkorn, M. Sigrist, P. Tregenna-Piggott, H. Mutka, H. Weihe, V. S. Mironov, J. Bendix, O. Waldmann,
Chem. Eur. J. 2013, 19, 3693.


11. An oxide-bridged Dy–ReV–Dy single-molecule magnet

K. S. Pedersen, J. Dreiser, M. Schau-Magnussen, C. Aa. Thuesen, H. Weihe, J. Bendix,
Polyhedron, 2012, 46, 47.


10. Fluoride-bridged {Ln2Cr2} polynuclear complexes from semi-labile mer-[CrF3(py)3] and [Ln(hfac)3(H2O)2]

C. Aa. Thuesen, K. S. Pedersen, M. Schau-Magnussen, M. Evangelisti, J. Vibenholt, S. Piligkos, H. Weihe, J. Bendix,
Dalton Trans. 2012, 41, 11284.


9. MnIII zero-field splitting parameters and weak exchange interactions in a cyanide-bridged {MnIII–IrIII–MnIII} cluster

K. S. Pedersen, M. Sigrist, H. Weihe, P. L. W. Tregenna-Piggott, M. Schau-Magnussen, J. Dreiser, H. Mutka, A.-L. Barra, J. Bendix,
Inorg. Chem. Commun. 2012, 24, 24.


8. X-ray Magnetic Circular Dichroism (XMCD) Study of a Methoxide-Bridged DyIII–CrIII Cluster Obtained by Fluoride Abstraction from cis-[CrIIIF2(phen)2]+

J. Dreiser, K. S. Pedersen, T. Birk, M. Schau-Magnussen, C. Piamonteze, S. Rusponi, T. Weyhermüller, H. Brune, F. Nolting, J. Bendix,
J. Phys. Chem. A, 2012, 116, 7842.


7. Fluoride Bridges as Structure Directing Motifs in 3d-4f Cluster Chemistry

T. Birk, K. S. Pedersen, C. Aa. Thuesen, T. Weyhermüller, M. Schau-Magnussen, S. Piligkos, S. Mossin, H. Weihe, M. Evangelisti, J. Bendix,
Inorg. Chem. 2012, 51, 5435.


6. Direct observation of a ferri-to-ferromagnetic transition in a fluoride-bridged 3d-4f molecular cluster

J. Dreiser, K. S. Pedersen, C. Piamonteze, S. Rusponi, Z. Salman, Md. E. Ali, M. Schau-Magnussen, C. Aa. Thuesen, S. Piligkos, H. Weihe,f H. Mutka, O. Waldmann, P. Oppeneer, J. Bendix, F. Nolting, H. Brune,
Chem. Sci. 2012, 3, 1024.


5. A linear single-molecule magnet based on [RuIII(CN)6]3–

K. S. Pedersen, J. Dreiser, J. Nehrkorn, M. Gysler, M. Schau-Magnussen, A. Schnegg, K. Holldack, R. Bittl, S. Piligkos, H. Weihe, P. Tregenna-Piggott, O. Waldmann, J. Bendix,
Chem. Commun. 2011, 47, 6918.


4. Magnetic Properties of a Manganese(III) Chain with Monoatomic Bridges: catena-MnF(salen)

T. Birk, K. S. Pedersen, S. Piligkos, C. Aa. Thuesen, H. Weihe, J. Bendix,
Inorg. Chem. 2011, 50, 5312.


3. Frequency-Domain Fourier-Transform Terahertz Spectroscopy of the Single-Molecule Magnet (NEt4)[Mn2(5-Brsalen)2(MeOH)2Cr(CN)6]

J. Dreiser, A. Schnegg, K. Holldack, K. S. Pedersen, M. Schau-Magnussen, J. Nehrkorn, P. Tregenna-Piggott, H. Mutka, H. Weihe, J. Bendix, O. Waldmann,
Chem. Eur. J. 2011, 17, 7492.


2. Enhancing the Blocking Temperature of Single-Molecule Magnets by Incorporating 3d-5d Exchange Interactions

K. S. Pedersen, M. Schau-Magnussen, J. Bendix, H. Weihe, A. V. Palii, S. I. Klokishner, S. M. Ostrovsky, O. S. Reu, H. Mutka, P. L. W. Tregenna-Piggott,
Chem. Eur. J. 2010, 16, 13458.


1. Single-Ion Anisotropy and Exchange Interactions in the Cyano-Bridged Trimers MnIII2MIII(CN)6 (MIII = Co, Cr, Fe) Species Incorporating [Mn(5-Brsalen)]+ Units: An Inelastic Neutron Scattering and Magnetic Susceptibility Study 

P. L. W. Tregenna-Piggott, D. Sheptyakov, L. Keller, S. I. Klokishner, S. M. Ostrovsky, A. V. Palii, O. S. Reu, J. Bendix, T. Brock-Nannestad, K. Pedersen, H. Weihe, H. Mutka,
Inorg. Chem. 2009, 48, 128.